| Record | Name | Role |
| ROLE125225 | Lang; Robert (1934-2004) | Martin Ruiz |
| ROLE125226 | Holder; Roy | Martin Ruiz, as a boy |
| ROLE125227 | Blakely; Colin | Francisco Pizarro, commander of the expedition |
| ROLE125228 | Turner; Michael | Hernando de Soto, second in command |
| ROLE125230 | Gambon; Sir; Michael | Diego de Trujillo, Master of Horse |
| ROLE125231 | Meaden; Dan | Salinas, blacksmith |
| ROLE125232 | Martin; Trevor | Rodas, tailor |
| ROLE125233 | Russell; Robert | Vasca |
| ROLE125234 | Kempinski; Tom | Domingo |
| ROLE125235 | Timothy; Christopher | Juan Chavez / Understudy: Rodas |
| ROLE125236 | Jacobi; Derek | Felipillo, an Indian boy employed as interpreter to Pizarro |
| ROLE125237 | Mackintosh; Kenneth | Fray Marcos de Nizza / Understudy: Hernando de Soto |
| ROLE125238 | Wylie; Frank | Pedro de Candia, commander of artillery |
| ROLE125239 | Cellier; Peter | Miguel Estete, royal overseer |
| ROLE125240 | Stephens; Robert (1931-1995) | Atahuallpa, soverign Inca of Peru |
| ROLE125241 | Petherbridge; Edward | Villac Umu, high priest of Peru / Understudy: Atahuallpa |
| ROLE125242 | Hardwicke; Edward | Challcuchima, a nobleman |
| ROLE125243 | Fitzpatrick; Neil | Manco / Messenger / Understudy: Fray Marcos de Nizza |
| ROLE125244 | John; Peter | Chieftain |
| ROLE125245 | Purchase; Bruce | Headman |
| ROLE125246 | Purnell; Louise (1942-) | Inti Coussi, step sister of Atahuallpa |
| ROLE125247 | John; Caroline | Oello, a wife of Atahuallpa |
| ROLE125248 | Byrne; Michael | Peruvian Indian / Understudy: Chieftain / Understudy: Villac / Understudy: Felipillo / Understudy: The Chieftain |
| ROLE125249 | Chittell; Christopher | Peruvian Indian |
| ROLE125250 | Edmett; Nicholas | Peruvian Indian |
| ROLE125251 | Knapp; Terence | Peruvian Indian |
| ROLE125252 | Pember; Ron | Peruvian Indian / Understudy: Domingo |
| ROLE125253 | Ridgway; Alan | Peruvian Indian |
| ROLE125254 | Rust; Clive | Peruvian Indian |
| ROLE125255 | Taylor; Pauline | Peruvian Indian |
| ROLE125256 | Curran; Paul | Francisco Pizarro, commaner of the expedition |
| ROLE125257 | Cellier; Peter | Fray Vincente de Valverde |
| ROLE125258 | Hallam; John | Salinas, blacksmith |
| ROLE125259 | Savident; John | Vasca |
| ROLE125260 | Pember; Ron | Domingo |
| ROLE125261 | Crowden; Graham | Miguel Estete, royal overseer |
| ROLE125262 | Byrne; Michael | Chieftain / Peruvian Indian |
| ROLE125263 | Ryall; David | Headman / Peruvian Indian |
| ROLE125272 | Ashcroft; Chloe | Peruvian Indian |
| ROLE125273 | Collins; Alan | Peruvian Indian |
| ROLE125274 | Gallie; Kay | Peruvian Indian |
| ROLE125276 | Jones; Carolyn | Peruvian Indian |
| ROLE125277 | Kemp; Roger | Peruvian Indian |
| ROLE125278 | Marne; Denis de | Peruvian Indian |
| ROLE125279 | Reynolds; Malcolm | Peruvian Indian |
| ROLE125281 | York; Michael | Peruvian Indian |
| ROLE125287 | Cotton; Oliver | Diego de Trujillo, Master of Horse |
| ROLE125288 | Pearce; Leonard | Salinas, blacksmith |
| ROLE125295 | Fitzpatrick; Neil | Fray Marcos de Nizza, Franciscan Friar |
| ROLE125298 | Reynolds; Malcolm | Manco |
| ROLE125301 | Adams; Alan | Peruvian Indian |
| ROLE125302 | Belcher; David | Peruvian Indian |
| ROLE125306 | McEnery; John | Peruvian Indian |
| ROLE140903 | McNally; Gerald | Pedro Chavez |
| ROLE140904 | Caddick; Edward | Fray Marcos de Nizza, Franciscan Friar |
| ROLE140906 | Christian; Kurt | Peruvian Indian |
| ROLE140907 | Darby; Anton | Peruvian Indian |
| ROLE140908 | Hobbs; William | Peruvian Indian |
| ROLE140909 | Rogers; John | Peruvian Indian |
| ROLE140917 | Kempinski; Tom | Rodas, tailor |
| ROLE140910 | Kempinski; Tom | Miguel Estete, royal overseer |
| ROLE140911 | Purchase; Bruce | Challcuchima, an Inca General |
| ROLE140912 | Rust; Clive | Headman |
| ROLE140913 | Heslewood; Jennie | Peruvian Indian |
| ROLE140914 | Pickup; Ronald | Peruvian Indian |
| ROLE140918 | Reynolds; Malcolm | Martin Ruiz, as a boy |
| ROLE140919 | Evans; Barry | Peruvian Indian |
| ROLE140920 | James; Gerald | Martin Ruiz |
| ROLE140921 | Timothy; Christopher | Rodas, tailor |
| ROLE140922 | Marne; Denis de | Vasca |
| ROLE140923 | Kemp; Roger | Juan Chavez |
| ROLE140924 | Hardy; Luke | Peruvian Indian |
| ROLE140925 | Mackintosh; Kenneth | Hernando de Soto, second in command |
| ROLE140926 | Bailie; David | Salinas, blacksmith |
| Reference Number | Title | Date | Series |
| RNT/PP/1/1/46 | The Royal Hunt of the Sun | 1966 | Pre-South Bank Programmes |
| RNT/PP/2/5/7 | The Royal Hunt of the Sun / A Flea in Her Ear | December 1966 | Repertory Posters |
| RNT/PP/5/4 | The Royal Hunt of the Sun | 1964 | Rehearsal Photographs |
| RNT/PP/1/1/59 | Much Ado About Nothing / The Royal Hunt of the Sun | November 1966 | Pre-South Bank Programmes |
| RNT/PP/1/1/47 | The Royal Hunt of the Sun | April 1967 | Pre-South Bank Programmes |
| RNT/PP/2/5/12 | The Royal Hunt of the Sun / A Flea in Her Ear | April 1967 | Repertory Posters |
| RNT/PR/3/11 | The Royal Hunt of the Sun | 1964 | Production Photographs |
| RNT/PP/1/1/48 | The Royal Hunt of the Sun | May 1967 | Pre-South Bank Programmes |
| CF/8/1 | The Royal Hunt of the Sun | 1964 | Scripts |
| RNT/PP/1/1/45 | The Royal Hunt of the Sun | 1964 | Pre-South Bank Programmes |
| RNT/PP/2/5/6 | Much Ado About Nothing / The Royal Hunt of the Sun / The Storm / A Flea in Her Ear / Love for Love | November 1966 | Repertory Posters |
| RNT/PP/2/5/14 | The Dance of Death / A Flea in Her Ear | May 1967 | Repertory Posters |
| RNT/PP/2/5/2 | Much Ado About Nothing / The Royal Hunt of the Sun | October 1966 | Repertory Posters |
| RNT/PP/2/5/3 | Much Ado About Nothing / The Royal Hunt of the Sun | November 1966 | Repertory Posters |
| RNT/PP/2/5/4 | Much Ado About Nothing / The Royal Hunt of the Sun | November 1966 | Repertory Posters |
| RNT/PP/2/5/13 | The Royal Hunt of the Sun / A Flea in Her Ear | May 1967 | Repertory Posters |
| RNT/PP/2/5/5 | Much Ado About Nothing / The Royal Hunt of the Sun / The Storm / A Flea in Her Ear / Love for Love | November 1966 | Repertory Posters |
| RNT/PP/3/6/4 | Much Ado About Nothing / The Royal Hunt of the Sun / The Storm / A Flea in her Ear / Love for Love | 1968 | Touring Printwork |
| RNT/R/1/4/3/117 | The Royal Hunt of the Sun | 1964 | Postcards |
| RNT/PP/3/6/9 | The Royal Hunt of the Sun | 1964 | Touring Printwork |
| RNT/LI/3/100 | The Royal Hunt of the Sun | 1964 | Scripts - Later Drafts |
| RNT/PP/3/6/10 | The Royal Hunt of the Sun / A Flea in Her Ear | 1966 - 1967 | Touring Printwork |
| RNT/PP/3/9/1/55g | The Royal Hunt of the Sun | 1964 | Old Vic Cast Lists |
| RNT/PP/1/6/5 | The Royal Hunt of the Sun | 05 December 1966 | Touring programmes |
| RNT/PP/1/6/3 | The Royal Hunt of the Sun | 12 August 1966 | Touring programmes |
| RNT/PP/1/6/7 | The Royal Hunt of the Sun | 1966 | Touring programmes |
| RNT/PP/2/5/1 | Much Ado About Nothing / The Royal Hunt of the Sun | October 1966 | Repertory Posters |
| RNT/SM/2/1/9 | The Royal Hunt of the Sun | 1 July 1964 - 29 June 1967 | Pre-South Bank Show Reports |
| RNT/PP/2/5/11 | The Royal Hunt of the Sun / A Flea in Her Ear | April 1967 | Repertory Posters |
| RNT/PP/2/5/8 | The Royal Hunt of the Sun / A Flea in Her Ear | December 1966 | Repertory Posters |
| RNT/SM/1/12 | The Royal Hunt of the Sun | 1964 | Prompt Scripts |
| RNT/PP/3/6/123 | Much Ado About Nothing / The Royal Hunt of the Sun | 1966 | Touring Printwork |
| RNT/PP/1/6/4 | Much Ado About Nothing / The Royal Hunt of the Sun | 07 November 1966 | Touring programmes |
| RNT/PP/3/9/1/55 | The Royal Hunt of the Sun | 1964 | Old Vic Cast Lists |
| RNT/PP/3/9/1/55b | The Royal Hunt of the Sun | 1964 | Old Vic Cast Lists |
| RNT/PP/3/9/1/55e | The Royal Hunt of the Sun | 1964 | Old Vic Cast Lists |
| RNT/PP/3/9/1/55d | The Royal Hunt of the Sun | 1964 | Old Vic Cast Lists |
| RNT/PP/3/9/1/55a | The Royal Hunt of the Sun | 1964 | Old Vic Cast Lists |
| RNT/PP/3/9/1/55c | The Royal Hunt of the Sun | 1964 | Old Vic Cast Lists |
| RNT/PP/3/9/1/55f | The Royal Hunt of the Sun | 1964 | Old Vic Cast Lists |
| RNT/PP/3/9/1/55h | The Royal Hunt for the Sun | 1964 | Old Vic Cast Lists |
| RNT/PP/1/1/44 | The Royal Hunt of the Sun | December 1964 | Pre-South Bank Programmes |
| RNT/PP/1/1/43 | The Royal Hunt of the Sun | December 1964 | Pre-South Bank Programmes |
| RNT/LI/3/314 | The Royal Hunt of the Sun | 1964 | Scripts - Later Drafts |
| RNT/PR/4/1/8 | The Royal Hunt of the Sun | December 1964 - January 1998 | Press Production Review Files |
| RNT/PP/2/1/2 | The Royal Hunt of the Sun | December 1964 | Pre-South Bank Posters |
| RNT/PP/2/1/3 | The Royal Hunt of the Sun | November 1966 | Pre-South Bank Posters |
| RNT/PP/2/1/4 | The Royal Hunt of the Sun | May 1967 | Pre-South Bank Posters |
| RNT/CO/1/11 | The Royal Hunt of the Sun | 1964 | Costume Department Production Files |
| RNT/PO/5/7 | The Royal Hunt of the Sun | 1964 | Set Photographs |